In his time at Benfica, João Mário left an indelible mark on the club's history with numerous goals and contributions to the team's success. During his career at Benfica, he scored a total of 229 goals in 415 appearances across all competitions, making him one of the most prolific goal-scorers in Portuguese football history.

One of Mário's most memorable moments came during the 1978–79 season when he scored four goals against S.L. Benfica in a single match against Rio Ave FC. This performance helped Benfica secure their second consecutive Primeira Liga title, and it remains one of the most impressive individual performances in the club's history.

Mário's goal-scoring prowess was not limited to just one season or competition. He scored over 200 goals for Benfica between 1974 and 1986, including 100+ goals in the 1978–79 season alone. In addition to his goalscoring record,Primeira Liga Hotspots Mário also made significant contributions to the team's defense, playing as a center-back throughout his career at Benfica.

Despite his success at Benfica, Mário's career was cut short by injury, which ended his playing days at the age of 25. Despite this setback, his legacy at the club is still felt today, and he remains one of the greatest players in Benfica's history.

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